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By Stuart A. Rice

This sequence presents the chemical physics box with a discussion board for severe, authoritative reviews of advances in each sector of the self-discipline. This stand-alone distinct subject matters quantity studies contemporary advances in electron-transfer learn with major, up to date chapters by means of the world over well-known researchers.

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Methods for solving the resulting equations are discussed in Section III. Section IV is devoted to a discussion of the Electric Nuclear Born–Oppenheimer (ENBO) approximation [41, 42]. This approximation provides a practical way of including polarization effects in coherent control calculations of molecular dynamics. In general, such effects are important as high electric fields often occur in the laser pulses used experimentally or predicted theoretically for such processes. The limits of validity of the ENBO approximation are also discussed in this section.

We also discuss an approach, with illustrative examples, for including effects beyond the dipole approximation and the use of analytic methods for guiding or interpreting OCT solutions. This chapter will not directly address any experimental problems. The interested reader is referred to the several excellent reviews focussing on the experimental aspects of control. [21–25]. Having said this, our general approach is that the theoretical treatment should be accurate and capable of correctly predicting and interpreting real experiments.

4, 2878 (2002). 76. E. J. Rackham, T. Gonzalez-Lezana, and D. E. Manolopoulos, J. Chem. Phys. 24, 12895 (2003). 77. M. Abe, Y. Ohtsuki, Y. Fujimura, Z. Lan, and W. Domcke, J. Chem. Phys. 124, 224316 (2006). OPTIMAL CONTROL THEORY FOR MANIPULATING MOLECULAR PROCESSES GABRIEL G. BALINT-KURTI and SHIYANG ZOU School of Chemistry, University of Bristol, Bristol BS8 1TS, UK ALEX BROWN Department of Chemistry, University of Alberta, Edmonton, AB, T6G 2G2, Canada CONTENTS I. Introduction II. Optimal Control Theory A.

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